Right click on Catalog -> Group Explorer -> right click on any smart group in the Explorer view -> Customize Column -> Enter 1 against the Name property, to sort by Name
You are looking for the same process using BLCLI commands?
My goal is to be able to expand on Windows OS Catalog, and all of the smartgroups will permanently be in alphabetical order.
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i believe it's in order of creation. you should open a ticket/defect for this.